Magneto-optical Faraday effect in spin-liquid candidates

Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. The MIT Faculty has made this article openly available. Please share how this access benefits you. Your story matters. We propose an experiment to use the magneto-optical Faraday effect to probe the dynamic Hall conductivity of spin-liquid candidates. Theory predicts that an external magnetic field will generate an internal gauge field. If the source of conductivity is in spinons with a Fermi surface, a finite Faraday rotation angle is expected. We predict the angle to scale as the square of the frequency rather than display the standard cyclotron resonance pattern. Furthermore, the Faraday effect should be able to distinguish the ground state of the spin liquid, as we predict no rotation for massless Dirac spinons. We give a semiquantitative estimate for the magnitude of the effect and find that it should be experimentally feasible to detect in both κ-(ET) 2 Cu 2 (CN) 3 and, if the spinons form a Fermi surface, herbertsmithite. We also comment on the magneto-optical Kerr effect and show that the imaginary part of the Kerr angle (circular dichroism) may be measurable.